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高电荷态类铍U88+, Th86+离子的同位素位移计算

Isotopic Shift of Be−like Highly Charged U88+, Th86+ Ions

  • 摘要: 利用相对论多组态Dirac-Hartree-Fock (MCDHF)方法计算了高电荷态类铍238U88+232Th86+离子的波函数以及 1s^22s^2 - 1s^22s2p ^1P_1的跃迁能。详细讨论了核反冲效应、Breit效应和量子电动力学(QED)效应(包括自能修正(SE)和真空极化(VP))对跃迁能的影响,深入研究了236U, 235U, 234, 233U, 230Th, 229Th, 228Th, 227Th的质量位移(MS)和场位移(FS)参数,并讨论了各项效应对于同位素位移(IS)的影响。目前的结果和已有实验、理论结果符合得都很好,其中跃迁能的计算精度达到了10−2 eV,IS的计算精度达到了10−2 meV。

     

    Abstract: The wavefunctions and eigenvalues of the 1s^22s^2-1s^22s2p ^1P_1 transitions for the highly charged ions 238U88+ and 232Th86+ were calculated using relativistic Multi-Configuration Dirac-Hartree-Fock (MCDHF) methods. The influence of nuclear recoil effects, the Breit effect, and quantum electrodynamics (QED) corrections — including self-energy (SE) and vacuum polarization (VP) — on transition energies is comprehensively analyzed. Additionally, mass shift and field shift parameters for isotopes 236U, 235U, 234U, 236U, 230Th, 229Th, 228Th, 227Th were also calculated, and the Contribution of each effect on the isotope shifts was thoroughly analyzed. The current results show good agreement with both experimental and theoretical data, with an accuracy within 10−2 eV in transition energy and within 10−2 meV in isotopic shifts.

     

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